FDTD MODELLING FOR ELECTROMAGNETIC FIELD ENHANCEMENT IN BOW-TIE ARRAY FOR SERS APPLICATIONS

Hasan Sarigul1, Tomas Tamulevičius1, 2

1 Department of Physics, Kaunas University of Technology, Studentų St. 50, Kaunas, LT-51368, Lithuania

2 Institute of Materials Science, Kaunas University of Technology, K. Baršausko St. 59, LT-51423, Kaunas, Lithuania

[email protected]

Surface-enhanced Raman Scattering (SERS) serves high-sensitivity technique for low-concentration and label-free detection of the fingerprint spectrum. SERS-based analyte sensing is attributed to the local electromagnetic (EM) field concentration, termed hotspots, that occur due to the gaps and edges between noble metal nanostructures [1]. Structures with nano-size gaps such as bow-tie geometries attract considerable attention from researchers as they can enhance EM fields significantly via plasmon coupling effects [2,3].

Since the SERS performance of noble metals is highly dependent on their geometry, we simulated the EM near fields in gold bow-tie triangle arrays employing the finite-difference time-domain (FDTD) method which is an effective computational method for examining nanostructures. The optical behavior of the edge sharpness and tip-to-tip gap parameters of the gold bow-tie triangle arrays were investigated. For the periodicity properties of the simulation region, boundary conditions were chosen as anti-symmetric for the X direction, symmetric for the Y direction, and perfectly matched layer (PML) for the Z direction. A 5 nm mesh was used for FDTD simulations the adjustments were made for the  785 nm resonant wavelengths. Optimization studies from sharp tips to 50 nm radius tips and nanogaps ranging from 0 to 200 nm showed that bow-tie structure with small nanogaps 5 nm, 10 nm, and 15 nm could enhance the incoming EM field intensity and SERS enhancement factor of approximately by up to 2.3 x 10\(^{3}\) and 3.9×10\(^{5}\), respectively. It was found that the gold bow-tie triangle array exhibits excellent SERS performance and significantly increases the EM field and SERS enhancement factor. This work was supported by the Research Council of Lithuania (RCL) (Project no.: S-PD-24-115).


[1] T. Gao et al., ACS Nano, vol. 18, no. 32, pp. 21593–21606,(2024).

[2] O. S. J. Hagger et al., Mater. Adv., vol. 4, no. 15, pp. 3239–3245, (2023).

[3] N. Khinevich et al., Sensors and Actuators B: Chemical, vol. 394, 134418, (2023).