ELECTROCHEMICAL ANALYSIS OF ENSIFER MELILOTI USING DIVERSE REDOX MEDIATORS FOR MFC APPLICATIONS

Asta Bubnelytė1, 2, Tomas Mockaitis2, Ingrida Bružaitė1, 2, Inga Morkvėnaitė-Vilkončienė2, 3

1 Department of Chemistry and Bioengineering, Faculty of Fundamental Sciences, Vilnius Gediminas Technical University, Vilnius 10223, Lithuania

2 Laboratory of Bioelectrochemical Technologies, Department of Nanotechnology, State Research Institute Centre for Physical Sciences and Technology, Vilnius 10257, Lithuania

3 Department of Electrical Engineering, Vilnius Gediminas Technical University, Vilnius 10223, Lithuania

[email protected]

As climate change intensifies and greenhouse gas emissions increase, there is growing global interest in finding sustainable solutions. A microbial fuel cell (MFC) is a bioelectrochemical system that can transform chemical energy into electrical energy, contributing to the reduction of pollution caused by harmful chemical compounds. This method emerged as a promising technology to address energy and environmental challenges by generating renewable energy [2].

Ensifer meliloti is a nitrogen-fixing bacterium that forms a symbiotic relationship with plants. The process begins when plant releases betaines and flavonoids that attract E. meliloti to root hairs. The bacteria then penetrate the root, forming nodules where they can develop into bacteroids, only then nitrogen fixation occur. Leghemoglobin, produced by the plant, regulates oxygen levels to maintain nitrogenase activity. These natural mechanisms could be adapted for microbial fuel cell [1]. MFCs utilize microbial catalysis to facilitate electron transfer, enhancing their efficiency in energy production. The use of redox mediators, such as quinones, is particularly significant, as they help improve electron flow between microbes and electrodes, advancing MFC performance. This mechanism makes MFCs a viable solution for clean energy generation while simultaneously addressing environmental concerns and reducing of pollutants [3].

This research aims to investigate the electrochemical behavior of Ensifer meliloti in microbial fuel cell while determining the efficiency of electron transfer and assessing its interaction with redox mediators, including various quinones and a K\(_{3}\)[Fe(CN)\(_{6}\)] solution.


[1] S. Bendinskaite, I. Bruzaite, J. Rožėnė, T. Mockaitis, I. Morkvenaite-Vilkonciene, A. Ramanaviciene, A. Zinovicius, & A. Ramanavicius. Microbial Fuel Cell Based on Ensifer meliloti. Journal of the Electrochemical Society, 171(10), (2024). https://doi.org/10.1149/1945-7111/ad8037.

[2] V. Reinikovaite, S. Zukauskas, R. Zalneravicius, V. Ratautaite, S. Ramanavicius, V. Bucinskas, M. Vilkiene, A. Ramanavicius, U. Samukaite Bubniene. Assessment of Rhizobium anhuiense Bacteria as a Potential Biocatalyst for Microbial Biofuel Cell Design. Biosensors, 13(1), (2023) https://doi.org/10.3390/bios13010066.

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