OPTICAL RESPONSE OF THE HYBRID TAMM-SURFACE PLASMON POLARITON MODES ON THE SURFACE LATTICE ARRAY OF GOLD NANO-BUMBS

Justina Anulytė1, Ernesta Bužavaitė-Vertelienė1, Vilius Vertelis1, Evaldas Stankevičius1, Kernius Vilkevičius1, Zigmas Balevičius1, 2

1 Plasmonics and nanophotonics lab., Department of Laser Technology, State research Institute Center for Physical Sciences and Technology, Saulėtekio ave. 3, LT-10257, Vilnius, Lithuania

2 Department of Computer Science and Communications Technologies, Faculty of Electronics, VilniusTech, Sauletekio ave. 11, LT-10223, Vilnius, Lithuania

[email protected]

Metallic nanostructures arranged in a periodic manner (grating arrays) have recently been used to reduce the losses in metal. Compared with the surface plasmon resonances or local surface plasmons in the randomly distributed metal nanoparticles, the metal nanoparticle lattices have a narrower plasmonic resonance [1]. Such periodic structures based nanophotonic – plasmonic devices have drawn attention to them due to various potential uses, such as plasmonic lasing [2] or enhanced bio-sensing [3], that may sustain prolonged coherence characteristics under the strong coupling. In this research two photonic-plasmonic structures (Fig. 1) that consist of 1D PC and either a thin gold layer (Fig. 1 b) or lattice of gold nano-bump (Fig. 1 c), supporting SPP and TPP modes, were investigated and compared. The strong coupling between the TPP and SPP were measured using the total internal reflection ellipsometry (TIRE) method.

Figure 1
Fig. 1. The investigate structure of PC/Au film (a) and PC/Au array (b) optical configuration and SEM micrograph of (c) a uniform (50 nm) Au layer and (d) a nano-bumps lattice array on the same thin gold layer [4].

According to recent research, the lattice of gold nano-bumps caused the development of an extra Bragg mode associated to the lattice period that was not strongly coupled to the hybrid TPP-SPP polaritonic mode. Despite this, the surface lattice-induced disturbance of the TPP and SPP components propagation length was discovered. Detailed study revealed that while the propagation length of the TPP reduced as a result of the emergence of an extra Bragg mode, the SPP's propagation length increased. The characteristics of 1D PC's optical dispersion and propagation with uniform gold layer and lattice of gold nano-bumps were evaluated by using a two linked oscillator's model and comparing broadening of the wave-vector vs. energy, allowing to indicate the degree of plasmonic modes field localization. The assessed propagation lengths for SPP and TPP components in hybrid polaritonic mode for nanostructures with homogeneous gold layers were $\delta_{SPP}$=5.5–6.5 μm and $\delta_{TPP}$=6.5–9.5 μm, respectively. In the meantime, the periodic gold surface lattice changes cause the propagation length of the SPP component (SPPlattice) to increase $\delta_{SPP_{lattice}}\approx$7-10.5 μm while the length of the TPP component (TPPlattice) decreases $\delta_{TPP_{lattice}}\sim$5.5-8.5 μm. The application of surface lattice resonances together with strong coupling regime leads to decreasing losses, resulting in the increasing propagation length and better coherence properties of such plasmonic resonances, which in turn promises advanced properties for threshold less plasmonic based coherent emission nano-sources [4].


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[2] Hakala T. K., Moilanen A. J., Väkeväinen et.al. Bose–Einstein condensation in a plasmonic lattice. Nat Phys 2018, 14(7),739–744.

[3] Paulauskas A., Tumenas S., Selskis A., et. al. Hybrid Tamm-surface plasmon polaritons mode for detection of mercury adsorption on 1D photonic crystal/gold nanostructures by total internal reflection ellipsometry. Opt Express 2018, 26(23), 30400.

[4] Anulyte J., Bužavaite-Verteliene E., Vertelis V. et. al. Influence of gold nano-bumps surface lattice array to the propagation lenght of strongly coupled Tamm and surface plasmon polariton, J. Mater. Chem. C, 2022, 10, 13234-13241.